Monday, April 8, 2013

Synthesis of La-substituted aluminosilicates with hierarchical pores by pH-adjusting method

Journal of Alloys and Compounds, Volume 557, 25 April 2013, Pages 223–227
Synthesis of La-substituted aluminosilicates with hierarchical pores by pH-adjusting method
Hongtao Liu, Jiujiang Wang, Wei Feng, Chunyan Xu
State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing 100029, PR China
Abstract
Researchers synthesized a novel La-containing hierarchical aluminosilicate (La-HA) from zeolite Y precursors using the pH-adjusting method. XRF showed that La-HA possessed a high La and Al loading.
TEM analysis suggested that La-HA displayed the ordered hexagonal arrays of uniform mesopores. N2 adsorptiondesorption revealed that the pore size and wall thickness of La-HA were greater than those of Al-HA. Diffuse reflectance UVvisible spectroscopy showed that La3+ was incorporated in the framework of the calcined materials. Such aluminosilicates show superior catalytic performance in heavy oil catalytic cracking.
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