Tuesday, October 22, 2013

Catalytic hydrotreatment in reverse microemulsions under microwave irradiation

CATEGORY: HYDROTREATMENT
Fuel, Volume 112, October 2013, Pages 338–346
Catalytic hydrotreatment in reverse microemulsions under microwave irradiation
Lorean Madriz (a), Hermes Carrero (a), José Ramón Domínguez (b), Ronald Vargas (c), Lenys Fernández (a)
a Universidad Simón Bolívar, Department of Chemistry, Laboratory of Electroanalysis, Apartado 89000, Caracas 1080A, Venezuela
b Universidad Simón Bolívar, Department of Chemistry, Laboratory of Spectroscopy, Apartado 89000, Caracas 1080A, Venezuela
c Universidad Simón Bolívar, Department of Chemistry, Laboratory of Electrochemistry, Apartado 89000, Caracas 1080A, Venezuela
Abstract
Reports a hydrocatalytic process developed in a reverse microemulsion using microwave irradiation. Researchers fabricated CoMo/Al2O3 and NiMo/Al2O3, in the laboratory. They analyzed the effectiveness of the procedure using such model compounds as nickel (II) phthalocyanine tetrasulfonate tetrasodium salt (NiPcTSNa4), nickel tetraphenylporphyrin (NiTPP) and thiophene.
They dematallized the first two model compounds to a percentage around 85% and 60% respectively. Desulfurization of the latter was greater than 90%. These values are higher than most of the values reported in the literature for this type of process. In addition, they applied this catalytic hydrotreating to an actual sample of Venezuelan heavy oil (Hamaca), achieving high conversion in a relatively short time. The results show the advantage of using this type of hydrotreating in less extreme conditions and in a shorter time than that used in other hydrocatalytic procedures.
Full Text Source (Subscription or Fee): http://www.sciencedirect.com/science/article/pii/S0016236113004328

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